Technical note: Isolating methane emissions from animal feeding operations in an interfering location

نویسندگان

چکیده

Abstract. Agricultural emissions, including those from concentrated animal feeding operations (CAFOs) for beef and dairy cattle, make up a large portion of the United States' total greenhouse gas (GHG) emissions. However, many CAFOs reside in areas where methane (CH4) oil natural (ONG) complicates quantification CAFO Traditional approaches to quantify emissions such regions often relied on inventory subtraction other known sources. We compare results two attribute CH4 emission rate derived an aircraft mass balance technique. These methods use mixing ratio data CH4, ethane (C2H6), ammonia (NH3) that were collected simultaneously in-flight downwind northeastern Colorado. The first approach, method (SM), is similar subtraction, except amount be removed observed C2H6 rather than estimate. this approach showed high uncertainty, primarily due how error propagates through subtraction. Alternatively, multivariate regression (MVR) can used estimate using NH3 ratio. significantly less uncertainty. identified criteria determine best attribution method; these support regions. final estimates presented here 13 ± 3 g per head hour 2 hour. are higher US Environmental Protection Agency (EPA) previous studies highlighting need more measurements rates.

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ژورنال

عنوان ژورنال: Atmospheric Chemistry and Physics

سال: 2023

ISSN: ['1680-7316', '1680-7324']

DOI: https://doi.org/10.5194/acp-23-7479-2023